Compiler optimization is essential for improving program performance, yet modern compilers still depend on manually crafted transformation rules over intermediate representations (IRs). As compilers grow in complexity, maintaining these rule-based optimizations becomes increasingly labor-intensive and difficult to scale. Recent advances in large language models (LLMs) offer a promising alternative, but their effectiveness in compiler optimization remains limited—primarily due to the lack of IR-oriented datasets that expose models to diverse transformation samples in real-world scenarios (optimization-sensitive samples), hindering LLMs from learning rich and generalizable optimization strategies.In this paper, we introduce IR-OptSet, the first public optimization-sensitive dataset for advancing LLM-based IR optimizers. It comprises 170K LLVM IR samples from open-source repositories across 8 representative optimization domains. IR-OptSet defines two core tasks: Code Analysis and Optimized Code Generation, and provides tools for correctness verification, performance evaluation, and dataset expansion. In our experiments, fine-tuning three representative LLMs on IR-OptSet leads to significant accuracy improvements across both tasks. Moreover, the LLM fine-tuned with IR-OptSet outperforms traditional compiler with the -O3 option in 64 test cases in terms of performance. Further analysis reveals that IR-OptSet provides greater transformation diversity and representativeness than three widely used IR-oriented datasets, highlighting its potential to drive model-based IR optimization. IR-OptSet is publicly available at https://huggingface.co/datasets/YangziResearch/IR-OptSet.

Compiler backends are tasked with generating executable machine code for processors. With the proliferation of diverse processors, it is imperative for programmers to tailor specific compiler backends to accommodate each one. Meanwhile, compiler backend development is a laborious and time-consuming task, lacking effective automation methods. Although language models have demonstrated strong abilities in code related tasks, the lack of appropriate datasets for compiler backend development limits the application of language models in this field.In this paper, we introduce ComBack, the first public dataset designed for improving compiler backend development capabilities of language models. ComBack includes 178 backends for mainstream compilers and three tasks including statement-level completion, next-statement suggestion and code generation, representing common development scenarios. We conducted experiments by fine-tuning six pre-trained language models with ComBack, demonstrating its effectiveness in enhancing model accuracy across the three tasks. We further evaluated the top-performing model(CodeT5+) across the three tasks for new targets, comparing its accuracy with conventional methods (Fork-Flow), ChatGPT-3.5-Turbo, and Code-LLaMA-34B-Instruct. Remarkably, fine-tuned CodeT5+ with only 220M parameters on ComBack outperformed Fork-Flow methods significantly and surpassed ChatGPT and Code-LLaMA. This suggests potential efficiency improvements in compiler development. ComBack is avaliable at https://huggingface.co/datasets/docz1105/ComBack.