This paper proposes a vector-quantization-based secret key generation (SKG) procedure to efficiently extract shared secret keys from correlated channel observations at two communicating terminals, Alice and Bob. Most existing SKG schemes utilize scalar quantization to extract secret key bits separately from each individual channel observation. This approach is simple to implement but yields higher key disagreement probability (or lower key entropy) compared with vector-quantization-based approaches. However, regardless of the quantizer design, quantization for SKG often suffers from the so-called cell-boundary problem, which occurs when the channel observations at Alice and Bob lie close to the quantization cell boundaries, resulting in high probability of key disagreement. In this paper, a general SKG procedure that utilizes sample and quantizer selection techniques to avoid this problem is first proposed. The vector quantizer adopted in the above procedure is designed by minimizing the quadratic distortion between the true channel vector and the noisy observation at Alice (or Bob). Then, by considering the case where the eavesdropper (Eve) may observe a channel vector that is correlated with that observed by Alice and Bob, a clustered key mapping scheme that assigns each secret key to multiple quantization cells in different clusters is also proposed to induce additional randomness at Eve and, thus, maintain high conditional key entropy. The effectiveness of the proposed schemes is demonstrated through computer simulations.