Concurrent measurements of atmospheric water vapor profiles were conducted over the Atlantic Ocean on September 25, 1995 with both the Millimeter-wave Imaging Radiometer (MIR) and Lidar Atmospheric Sounding Experiment (LASE) on board the NASA ER-2 aircraft. LASE provides high precision measurements of both aerosol backscatter and water vapor profiles; aerosol backscatter has a vertical resolution of 60 m while the water vapor profiles have a resolution of 330 m in the low-to-mid troposphere and 550 m in the upper troposphere. Therefore, LASE measurements provide an excellent resource for assessing the capabilities and limitations of MIR as a water vapor profiler. Previously, the water vapor profiles retrieved from the MIR measurements have been compared with those of rawinsonde and Raman lidar observations at point locations. The frequency and extent of the comparisons made in that fashion were largely constrained by the requirement of near coincidence in time and space. The data acquired concurrently by MIR and LASE from this ER-2 aircraft flight enable the comparison of MIR-retrieved and LASE-measured moisture profiles over a long stretch of time and space. In addition, the LASE-measured profiles of aerosol backscatter provide a resource to assess the impact of clouds on the retrieval of water vapor profiles from the MIR measurements. It is shown that profiles of water vapor mixing ratio retrieved from the MIR data generally conform to those measured by the LASE; however, differences in the values of mixing ratio at individual altitude levels are quite often not small. The standard deviations of these differences are found to be about. /spl plusmn/0.98, /spl plusmn/0.84, /spl plusmn/0.95, /spl plusmn/0.42, and /spl plusmn/0.06 g/kg at altitudes of 1.25, 2.75, 4.75, 7.25, and 10.25 km. It is demonstrated that a substantial portion of these differences are due to the poor vertical resolution inherent in the profile retrieval using the MIR radiometric measurements. Additionally, MIR water vapor profiling under cloudy conditions is demonstrated, and it is shown that location and height of the low-altitude clouds estimated from the retrieval process were generally consistent with those observed by the LASE. For study cases where cirrus clouds are present, retrievals from the MIR data over-estimate the mixing ratio; this over-estimate is provoked by brightness temperature decreases that occur at 183-220 GHz within these regions. Undoubtedly, the retrieval method needs an additional procedure to account for the mm-wave scattering by cloud ice particles so that water vapor profiling can be improved within regions where cirrus clouds are present.

The differential absorption lidar (DIAL) technique for deriving O/sub 3/ profiles from lidar measurements is discussed. The US National Aeronautics and Space Administration's airborne DIAL system is described, and examples of a broad range of O/sub 3/ and aerosol measurements are presented from a number of field experiments. The airborne and ground-based DIAL measurements discussed demonstrate the outstanding capability of lidar for conducting O/sub 3/ investigations throughout the troposphere and lower stratosphere under widely different atmospheric conditions.>