We exhibit infinitely many new, constrained inequalities for the von Neumann entropy, and show that they are independent of each other and the known inequalities obeyed by the von Neumann entropy (basically strong subadditivity). The new inequalities were proved originally by Makarychevfor the Shannon entropy, using properties of probability distributions. Our approach extends the proof of the inequalities to the quantum domain, and includes their independence for the quantum and also the classical cases.